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[1]馬彩霞,劉蕾,李碧清,等.強(qiáng)化化學(xué)淋濾對污泥重金屬溶出及磷釋放的影響[J].中國給水排水,2021,37(5):66-70.
MA Cai-xia,LIU Lei,LI Bi-qing,et al.Effect of Enhanced Chemical Leaching on Heavy Metal Dissolution and Phosphorus Release from Sludge[J].China Water & Wastewater,2021,37(5):66-70.點(diǎn)擊復(fù)制
強(qiáng)化化學(xué)淋濾對污泥重金屬溶出及磷釋放的影響
中國給水排水[ISSN:1000-4062/CN:12-1073/TU] 卷: 第37卷 期數(shù): 2021年第5期 頁碼: 66-70 欄目: 出版日期: 2021-03-01
Title:Effect of Enhanced Chemical Leaching on Heavy Metal Dissolution and Phosphorus Release from Sludge
作者:馬彩霞1,2，劉蕾3，李碧清4，李鵬飛4，肖羽堂1,2，張立國1,2(1.華南師范大學(xué)環(huán)境學(xué)院廣東省化學(xué)品污染與環(huán)境安全重點(diǎn)實(shí)驗室，廣東廣州510006；2.華南師范大學(xué)環(huán)境學(xué)院教育部環(huán)境理論化學(xué)重點(diǎn)實(shí)驗室，廣東廣州510006；3.東莞理工學(xué)院生態(tài)環(huán)境與建筑工程學(xué)院，廣東東莞523808；4.廣州市凈水有限公司，廣東廣州510163)
Author(s):MA Cai-xia1,2，LIU Lei3，LI Bi-qing4，LI Peng-fei4，XIAO Yu-tang1,2，ZHANG Li-guo1,2(1. Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety, School of Environment, South China Normal University, Guangzhou 510006， China; 2. Key Laboratory of Theoretical Chemistry of Environment ， School of Environment, South China Normal University, Guangzhou 510006， China; 3. School of Environment and Civil Engineering, Dongguan University of Technology, Dongguan 523808， China; 4. Guangzhou Sewage Purification Co. Ltd.， Guangzhou 510163， China)
關(guān)鍵詞:污泥; 重金屬溶出; 磷釋放; 脫水性
Keywords:sludge; dissolution of heavy metals; phosphorus release; dewaterability
摘要:針對采用傳統(tǒng)化學(xué)淋濾方法處理污水污泥時重金屬溶出率低的問題，設(shè)計了兩種強(qiáng)化化學(xué)淋濾方法的對比試驗，通過檢測重金屬形態(tài)分布、污泥有機(jī)質(zhì)及磷釋放、污泥含固率，研究了強(qiáng)化化學(xué)淋濾對污泥各方面綜合性能的影響。結(jié)果表明：稀硫酸與氯化鐵聯(lián)合處理（處理方法1）對Cu和Cr的溶出效果不明顯，但在加入NaNO2（處理方法2）后使Cu溶出率由7%提升至82%，Zn溶出率由79%提升至88%；同時，兩種強(qiáng)化化學(xué)淋濾方法均增加了污泥中有機(jī)質(zhì)和磷的釋放，污泥中磷含量由23.2 mg/g分別降至12.3 mg/g和10.7 mg/g；與原污泥相比，強(qiáng)化淋濾后的污泥脫水性也均得到了明顯改善，其污泥含固率分別提高了52％和61％。
Abstract:In order to solve the problem of low dissolution rate of heavy metals when using traditional chemical leaching method to treat sewage sludge, contrastive tests of two enhanced chemical leaching methods were designed, and effects of enhanced chemical leaching on comprehensive properties of the treated sludge were explored through determination of heavy metal speciation distribution, sludge organic matters and phosphorus release and sludge solids content. The combined treatment of dilute sulfuric acid and ferric chloride (method 1) had no obvious effect on Cu and Cr dissolution, however, the addition of NaNO2 (method 2) could enhance the Cu dissolution rate from 7% to 82% and the Zn dissolution rate from 79% to 88%. Meanwhile, both methods increased the release of organic matters and phosphorus in sludge, and the phosphorus contents decreased from 23.2 mg/g to 12.3 mg/g and 10.7 mg/g, respectively. Compared with the raw sludge, dewaterability of the enhanced leaching sludge was also improved obviously, and solid contents of the sludge increased by 52% and 61%, respectively.
相似文獻(xiàn)/References:
[1]劉常青,陳琬,曾藝芳,等.SARD與CSTR反應(yīng)器半連續(xù)發(fā)酵產(chǎn)氫能力對比[J].中國給水排水,2018,34(21):7.
LIU Chang qing,CHEN Wan,ZENG Yi fang,et al.Hydrogen Production Capacity of Semi continuous Fermentation of SARD and CSTR Bio hydrogen Production Reactor[J].China Water & Wastewater,2018,34(5):7.
[2]顏瑩瑩,梁遠(yuǎn),沙雪華,等.新冠肺炎疫情下關(guān)于減少污泥中病原體的思考[J].中國給水排水,2020,36(6):22.
[3]郭波,田瑜,范晨,等.綠色納米鐵/H2O2聯(lián)用兩性脫水劑調(diào)理污泥研究[J].中國給水排水,2020,36(13):62.
GUO Bo,TIAN Yu,FAN Chen,et al. Sludge Conditioning by Green Iron Nanoparticles/H2O2 Combined with Amphoteric Dewatering Agent [J].China Water & Wastewater,2020,36(5):62.
[4]許勁,范準(zhǔn),呂秋穎,等.山地城市污泥水熱炭化產(chǎn)物特性研究[J].中國給水排水,2020,36(21):21.
XU Jin,FAN Zhun,L Qiu-ying,et al.Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in Mountainous Cities[J].China Water & Wastewater,2020,36(5):21.
[5]李金河,張波濤,劉寶玉,等.污泥中溫厭氧消化最佳溫度及改善機(jī)理分析[J].中國給水排水,2021,37(3):9.
LI Jin-he,ZHANG Bo-tao,LIU Bao-yu,et al.Optimal Reaction Temperature in Mesophilic Anaerobic Digestion of Waste Activated Sludge and Its Promotion Mechanism[J].China Water & Wastewater,2021,37(5):9.
[6]王麗花,呂國鈞,王飛,等.污泥干化焚燒系統(tǒng)的節(jié)能降耗研究[J].中國給水排水,2021,37(4):29.
WANG Li-hua,Lü Guo-jun,WANG Fei,et al.Research on Energy Saving and Consumption Reduction of Sludge Drying and Incineration System[J].China Water & Wastewater,2021,37(5):29.
[7]紀(jì)莎莎,黃瑾.污泥焚燒工程中的磷形態(tài)分布與磷遷移研究[J].中國給水排水,2021,37(5):26.
JI Sha-sha,HUANG Jin.Phosphorus Forms Distribution and Migration in Sludge Incineration Project[J].China Water & Wastewater,2021,37(5):26.
[8]李偉,常菁,王佳偉,等.熱水解高級厭氧消化系統(tǒng)的污泥消毒、減量與能量回收[J].中國給水排水,2021,37(16):19.
LI Wei,CHANG Jing,WANG Jia-wei,et al.Sludge Disinfection, Reduction and Energy Recovery by Anaerobic Digestion with Thermal Hydrolysis Pretreatment[J].China Water & Wastewater,2021,37(5):19.
[9]胡佩佩,侯鋒,范瑩,等.深度脫水污泥好氧發(fā)酵工藝研究[J].中國給水排水,2021,37(17):74.
HU Pei-pei,HOU Feng,FAN Ying,et al.Aerobic Fermentation Process of Deep Dewatering Sludge[J].China Water & Wastewater,2021,37(5):74.
[10]齊利格娃,李偉,高金華,等.污泥高含固厭氧消化研究進(jìn)展[J].中國給水排水,2021,37(18):14.
QI Li-ge-wa,LI Wei,GAO Jin-hua,et al.Research Progress on High-solids Anaerobic Digestion of Sewage Sludge[J].China Water & Wastewater,2021,37(5):14.
更新日期/Last Update: 2021-03-01
[1]馬彩霞,劉蕾,李碧清,等.強(qiáng)化化學(xué)淋濾對污泥重金屬溶出及磷釋放的影響[J].中國給水排水,2021,37(5):66-70.
MA Cai-xia,LIU Lei,LI Bi-qing,et al.Effect of Enhanced Chemical Leaching on Heavy Metal Dissolution and Phosphorus Release from Sludge[J].China Water & Wastewater,2021,37(5):66-70.
點(diǎn)擊復(fù)制
強(qiáng)化化學(xué)淋濾對污泥重金屬溶出及磷釋放的影響
中國給水排水[ISSN:1000-4062/CN:12-1073/TU] 卷: 第37卷 期數(shù): 2021年第5期 頁碼: 66-70 欄目: 出版日期: 2021-03-01
- Title:
- Effect of Enhanced Chemical Leaching on Heavy Metal Dissolution and Phosphorus Release from Sludge
- 作者:
- 馬彩霞1,2，劉蕾3，李碧清4，李鵬飛4，肖羽堂1,2，張立國1,2
- (1.華南師范大學(xué)環(huán)境學(xué)院廣東省化學(xué)品污染與環(huán)境安全重點(diǎn)實(shí)驗室，廣東廣州510006；2.華南師范大學(xué)環(huán)境學(xué)院教育部環(huán)境理論化學(xué)重點(diǎn)實(shí)驗室，廣東廣州510006；3.東莞理工學(xué)院生態(tài)環(huán)境與建筑工程學(xué)院，廣東東莞523808；4.廣州市凈水有限公司，廣東廣州510163)
Author(s):- MA Cai-xia1,2，LIU Lei3，LI Bi-qing4，LI Peng-fei4，XIAO Yu-tang1,2，ZHANG Li-guo1,2
- (1. Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety, School of Environment, South China Normal University, Guangzhou 510006， China; 2. Key Laboratory of Theoretical Chemistry of Environment ， School of Environment, South China Normal University, Guangzhou 510006， China; 3. School of Environment and Civil Engineering, Dongguan University of Technology, Dongguan 523808， China; 4. Guangzhou Sewage Purification Co. Ltd.， Guangzhou 510163， China)
- 關(guān)鍵詞:
- 污泥; 重金屬溶出; 磷釋放; 脫水性
- Keywords:
- sludge; dissolution of heavy metals; phosphorus release; dewaterability
摘要:- 針對采用傳統(tǒng)化學(xué)淋濾方法處理污水污泥時重金屬溶出率低的問題，設(shè)計了兩種強(qiáng)化化學(xué)淋濾方法的對比試驗，通過檢測重金屬形態(tài)分布、污泥有機(jī)質(zhì)及磷釋放、污泥含固率，研究了強(qiáng)化化學(xué)淋濾對污泥各方面綜合性能的影響。結(jié)果表明：稀硫酸與氯化鐵聯(lián)合處理（處理方法1）對Cu和Cr的溶出效果不明顯，但在加入NaNO2（處理方法2）后使Cu溶出率由7%提升至82%，Zn溶出率由79%提升至88%；同時，兩種強(qiáng)化化學(xué)淋濾方法均增加了污泥中有機(jī)質(zhì)和磷的釋放，污泥中磷含量由23.2 mg/g分別降至12.3 mg/g和10.7 mg/g；與原污泥相比，強(qiáng)化淋濾后的污泥脫水性也均得到了明顯改善，其污泥含固率分別提高了52％和61％。
Abstract:- In order to solve the problem of low dissolution rate of heavy metals when using traditional chemical leaching method to treat sewage sludge, contrastive tests of two enhanced chemical leaching methods were designed, and effects of enhanced chemical leaching on comprehensive properties of the treated sludge were explored through determination of heavy metal speciation distribution, sludge organic matters and phosphorus release and sludge solids content. The combined treatment of dilute sulfuric acid and ferric chloride (method 1) had no obvious effect on Cu and Cr dissolution, however, the addition of NaNO2 (method 2) could enhance the Cu dissolution rate from 7% to 82% and the Zn dissolution rate from 79% to 88%. Meanwhile, both methods increased the release of organic matters and phosphorus in sludge, and the phosphorus contents decreased from 23.2 mg/g to 12.3 mg/g and 10.7 mg/g, respectively. Compared with the raw sludge, dewaterability of the enhanced leaching sludge was also improved obviously, and solid contents of the sludge increased by 52% and 61%, respectively.
相似文獻(xiàn)/References:
[1]劉常青,陳琬,曾藝芳,等.SARD與CSTR反應(yīng)器半連續(xù)發(fā)酵產(chǎn)氫能力對比[J].中國給水排水,2018,34(21):7.
LIU Chang qing,CHEN Wan,ZENG Yi fang,et al.Hydrogen Production Capacity of Semi continuous Fermentation of SARD and CSTR Bio hydrogen Production Reactor[J].China Water & Wastewater,2018,34(5):7.
[2]顏瑩瑩,梁遠(yuǎn),沙雪華,等.新冠肺炎疫情下關(guān)于減少污泥中病原體的思考[J].中國給水排水,2020,36(6):22.
[3]郭波,田瑜,范晨,等.綠色納米鐵/H2O2聯(lián)用兩性脫水劑調(diào)理污泥研究[J].中國給水排水,2020,36(13):62.
GUO Bo,TIAN Yu,FAN Chen,et al. Sludge Conditioning by Green Iron Nanoparticles/H2O2 Combined with Amphoteric Dewatering Agent [J].China Water & Wastewater,2020,36(5):62.
[4]許勁,范準(zhǔn),呂秋穎,等.山地城市污泥水熱炭化產(chǎn)物特性研究[J].中國給水排水,2020,36(21):21.
XU Jin,FAN Zhun,L Qiu-ying,et al.Characteristics of Hydrothermal Carbonization Products of Municipal Sludge in Mountainous Cities[J].China Water & Wastewater,2020,36(5):21.
[5]李金河,張波濤,劉寶玉,等.污泥中溫厭氧消化最佳溫度及改善機(jī)理分析[J].中國給水排水,2021,37(3):9.
LI Jin-he,ZHANG Bo-tao,LIU Bao-yu,et al.Optimal Reaction Temperature in Mesophilic Anaerobic Digestion of Waste Activated Sludge and Its Promotion Mechanism[J].China Water & Wastewater,2021,37(5):9.
[6]王麗花,呂國鈞,王飛,等.污泥干化焚燒系統(tǒng)的節(jié)能降耗研究[J].中國給水排水,2021,37(4):29.
WANG Li-hua,Lü Guo-jun,WANG Fei,et al.Research on Energy Saving and Consumption Reduction of Sludge Drying and Incineration System[J].China Water & Wastewater,2021,37(5):29.
[7]紀(jì)莎莎,黃瑾.污泥焚燒工程中的磷形態(tài)分布與磷遷移研究[J].中國給水排水,2021,37(5):26.
JI Sha-sha,HUANG Jin.Phosphorus Forms Distribution and Migration in Sludge Incineration Project[J].China Water & Wastewater,2021,37(5):26.
[8]李偉,常菁,王佳偉,等.熱水解高級厭氧消化系統(tǒng)的污泥消毒、減量與能量回收[J].中國給水排水,2021,37(16):19.
LI Wei,CHANG Jing,WANG Jia-wei,et al.Sludge Disinfection, Reduction and Energy Recovery by Anaerobic Digestion with Thermal Hydrolysis Pretreatment[J].China Water & Wastewater,2021,37(5):19.
[9]胡佩佩,侯鋒,范瑩,等.深度脫水污泥好氧發(fā)酵工藝研究[J].中國給水排水,2021,37(17):74.
HU Pei-pei,HOU Feng,FAN Ying,et al.Aerobic Fermentation Process of Deep Dewatering Sludge[J].China Water & Wastewater,2021,37(5):74.
[10]齊利格娃,李偉,高金華,等.污泥高含固厭氧消化研究進(jìn)展[J].中國給水排水,2021,37(18):14.
QI Li-ge-wa,LI Wei,GAO Jin-hua,et al.Research Progress on High-solids Anaerobic Digestion of Sewage Sludge[J].China Water & Wastewater,2021,37(5):14.
更新日期/Last Update: 2021-03-01
